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research article

Singlet state formation and its impact on the magnetic structure in the tetramer system SeCuO3

Cvitanić, Tonči
•
Šurija, Vinko
•
Prša, Krunoslav
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2018
Physical Review B

We present an experimental investigation of the magnetic structure in a tetramer system SeCuO3 using neutron powder-diffraction and nuclear resonance techniques. We establish a commensurate antiferromagnetic ordering with a propagation vector k = (0, 0, 1). The order parameter follows a critical behavior near T-N = 8 K with a critical exponent beta = 0.32 in agreement with a three-dimensional universality class. Evidence is presented that a singlet state starts to form on tetramers at temperatures as high as 200 K, and its signature is preserved within the ordered state through a strong renormalization of the ordered magnetic moment on two nonequivalent copper sites m(Cu1) approximate to 0.35(mu B) and m(Cu2) < 0.8(mu B) at 1.5 K.

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Type
research article
DOI
10.1103/PhysRevB.98.054409
Author(s)
Cvitanić, Tonči
Šurija, Vinko
Prša, Krunoslav
Zaharko, Oksana
Kupčić, Ivan
Babkevich, Peter
Frontzek, Matthias
Požek, Miroslav
Berger, Helmuth
Magrez, Arnaud
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Date Issued

2018

Published in
Physical Review B
Volume

98

Issue

5

Article Number

054409

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
FunderGrant Number

FNS

166298

FNS

169699

Available on Infoscience
October 12, 2018
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/148813
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