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  4. Electrodeposition of polyaniline on reduced graphene oxide/cotton yarn with tunable electrochemical performance for flexible textile supercapacitors
 
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research article

Electrodeposition of polyaniline on reduced graphene oxide/cotton yarn with tunable electrochemical performance for flexible textile supercapacitors

Li, Lin
•
Du, Dou  
•
He, Chengen
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June 21, 2024
Polymer

Graphene/cotton fibers show significant promise in wearable energy storage due to their low cost, porous structure, and exceptional integration ability into wearable systems. However, the eco-unfriendly reductants and standalone electric double-layer capacitor hindered their application. Herein, a green and rapid hydrothermal-electrodeposition method was proposed to fabricate polyaniline (PANI) decorated reduced graphene oxide (rGO)/cotton yarns without using any chemical reductants and oxidants. The PANI/rGO/cotton (PRC) yarn exhibited porous conductive network, structural controllability, and mechanical flexibility. Additionally, the PRC yarn electrode delivers a fast electron transport and ion migration, synergistic energy storage contribution, and a controllable capacitance (up to 81.2 mF cm(-1) at 0.2 mA cm(-1)). The assembled yarn supercapacitor shows a good capacitance (19.8 mF cm(-1) at 0.08 mA cm(-1)), excellent energy-power density (2.7 mu Wh cm(-1) at 40 mu W cm(-1)), and great capacitance retention. This green fabrication of PRC yarns brings new insights into the development of wearable energy storage.

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Type
research article
DOI
10.1016/j.polymer.2024.127200
Web of Science ID

WOS:001254279900002

Author(s)
Li, Lin
•
Du, Dou  
•
He, Chengen
•
Han, Kun
•
Xu, Weilin
•
Xia, Liangjun
•
Cai, Guangming
•
Cui, Xun
•
Chen, Yihuang
•
Yu, Lianqing
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Date Issued

2024-06-21

Publisher

Elsevier Sci Ltd

Published in
Polymer
Volume

306

Article Number

127200

Subjects

Physical Sciences

•

Flexible Textile Supercapacitor

•

Tunable Electrochemical Performance

•

Pani

•

Rgo

•

Electrodeposition

Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
THEOS  
FunderGrant Number

National Natural Science Foundation of China

52003207

Foundation of Science Research Program from the Hubei Provincial Department of Education

Q20211706

Open foundation of the Key Laboratory of Catalysis and Energy Materials Chemistry of Ministry of Education & Hubei Key Laboratory of Catalysis and Materials Science

CHCL21006

Available on Infoscience
July 3, 2024
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/209174
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