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  4. Low Current Density Driving Leads to Efficient, Bright, and Stable Green Electroluminescence
 
research article

Low Current Density Driving Leads to Efficient, Bright, and Stable Green Electroluminescence

Tordera, Daniel
•
Frey, Julien  
•
Vonlanthen, David
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2013
Advanced Energy Materials

Electroluminescent devices have the potential to reshape lighting and display technologies by providing low-energy consuming solutions with great aesthetic features, such as flexibility and transparency. In particular, light-emitting electrochemical cells (LECs) are among the simplest electro-luminescent devices. The device operates with air-stable materials and the active layer can be resumed to an ionic phosphorescent emitter. As a consequence, LECs can be assembled using solution-process technologies, which could allow for low-cost and large-area lighting applications in the future. High efficiencies have been reported at rather low luminances (<50 cd m(-2)) and at very low current densities. Moreover, these efficiencies could be sustained for a brief moment only during operation time. Here, we demonstrate that a pulsed driving mode at low current densities leads to unequalled overall performances with excellent efficiencies throughout the lifetime of the device. The lifetime of the LECs is defined as the time it takes to reach 50% of the peak luminance. Upon optimization of various parameters (frequency, duty cycle and average current density), the green LEC reaches efficacies and power efficiencies of 28.2 cd A(-1) and 17.1 lm W-1, respectively, at a luminance above 750 cd m(-2) and 98 hours lifetime. The present work also rationalizes why high efficiencies have been obtained only at low current densities so far.

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Type
research article
DOI
10.1002/aenm.201300284
Web of Science ID

WOS:000328742200013

Author(s)
Tordera, Daniel
Frey, Julien  
Vonlanthen, David
Constable, Edwin
Pertegas, Antonio
Orti, Enrique
Bolink, Henk J.
Baranoff, Etienne  
Nazeeruddin, M. Khaja  
Date Issued

2013

Publisher

Wiley-VCH Verlag Berlin

Published in
Advanced Energy Materials
Volume

3

Issue

10

Start page

1338

End page

1343

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LPI  
Available on Infoscience
January 20, 2014
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/100004
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