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  4. Disclosing the response of the surface electronic structure in SrTiO3 (001) to strain
 
research article

Disclosing the response of the surface electronic structure in SrTiO3 (001) to strain

Guedes, Eduardo Bonini
•
Jensen, Tobias Willemoes
•
Naamneh, Muntaser
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January 1, 2022
Journal Of Vacuum Science & Technology A

Combining angle-resolved photoemission spectroscopy and density functional theory calculations, we addressed the surface electronic structure of bent SrTiO 3 (STO) (001) wafers. Using a custom-made device, we observe that the low-dimensional states that emerge at the STO (001) surface are robust to an external tensile strain of about 0.1%. Our results show that this value of strain is too small to sensibly alter the surface conduction band of STO, but, surprisingly, it is enough to shift the energy of the in-gap states. In order to access higher strain values of around 2%, standard for STO-based heterostructures, we performed density functional theory calculations of STO slabs under different strain configurations. The simulations predict that such levels of both compressive and tensile strain significantly alter the orbital splitting of the surface conduction band. Our study indicates that the strain generated in STO can tailor the electronic properties of its bare surface and of STO-based interfaces.

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Type
research article
DOI
10.1116/6.0001480
Web of Science ID

WOS:000732534000002

Author(s)
Guedes, Eduardo Bonini
Jensen, Tobias Willemoes
Naamneh, Muntaser
Chikina, Alla
Dahm, Ramus T.
Yun, Shinhee
Chiabrera, Francesco M.
Plumb, Nicholas C.
Dil, J. Hugo  
Shi, Ming
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Date Issued

2022-01-01

Published in
Journal Of Vacuum Science & Technology A
Volume

40

Issue

1

Article Number

013213

Subjects

Materials Science, Coatings & Films

•

Physics, Applied

•

Materials Science

•

Physics

•

total-energy calculations

•

insulator-transition

•

gas

•

oxides

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
SCI-SB-HD  
Available on Infoscience
January 31, 2022
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/185014
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