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research article

Performance of perovskite solar cells under simulated temperature-illumination real-world operating conditions

Tress, Wolfgang  
•
Domanski, Konrad  
•
Carlsen, Brian  
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July 1, 2019
Nature Energy

Since reaching 20% efficiency, research in perovskite photovoltaics has shifted from a race for efficiency to a race for stability. For efficiency, the standard test conditions set the rules for the race. However, the term 'stability' is used very broadly and assessed in various ways, meaning different groups are running different races. For the application, only energy yields that can be achieved under real-world, long-term operation matter. Here, we characterize and analyse the performance of an efficient perovskite solar cell (PSC) under simulated ambient conditions based on real temperature and irradiance data from selected days over one year at a location in central Europe. We find that the PSC shows only a low decrease of efficiency with elevated temperature and low light intensity, maintaining almost optimum values for ambient conditions, under which most of the solar energy is incident on the solar cell. The overall energy yield differs from what is expected from standard test condition measurements and is influenced by reversible degradation (delivering the highest performance in the morning) and by a slight permanent degradation that is observable during the year. With reference to tandem cells, we compare the PSC with a silicon device.

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Type
research article
DOI
10.1038/s41560-019-0400-8
Web of Science ID

WOS:000474920100013

Author(s)
Tress, Wolfgang  
Domanski, Konrad  
Carlsen, Brian  
Agarwalla, Anand  
Alharbi, Essa A.  
Graetzel, Michael  
Hagfeldt, Anders  
Date Issued

2019-07-01

Publisher

NATURE PUBLISHING GROUP

Published in
Nature Energy
Volume

4

Issue

7

Start page

568

End page

574

Subjects

Energy & Fuels

•

Materials Science, Multidisciplinary

•

Energy & Fuels

•

Materials Science

•

outdoor performance

•

hole transport

•

light-soaking

•

stability

•

degradation

•

dependence

•

efficiency

•

migration

•

behavior

•

cations

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSPM  
LPI  
Available on Infoscience
July 24, 2019
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/159311
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