Repository logo

Infoscience

  • English
  • French
Log In
Logo EPFL, École polytechnique fédérale de Lausanne

Infoscience

  • English
  • French
Log In
  1. Home
  2. Academic and Research Output
  3. Journal articles
  4. Low-temperature solution-processed wavelength-tunable perovskites for lasing
 
research article

Low-temperature solution-processed wavelength-tunable perovskites for lasing

Xing, Guichuan
•
Mathews, Nripan
•
Lim, Swee Sien
Show more
2014
Nature Materials

Low-temperature solution-processed materials that show optical gain and can be embedded into a wide range of cavity resonators are attractive for the realization of on-chip coherent light sources. Organic semiconductors and colloidal quantum dots are considered the main candidates for this application. However, stumbling blocks in organic lasing(1-4) include intrinsic losses from bimolecular annihilation and the conflicting requirements of high charge carrier mobility and large stimulated emission; whereas challenges pertaining to Auger losses and charge transport in quantum dots(5-7) still remain. Herein, we reveal that solution-processed organic-inorganic halide perovskites (CH3NH3PbX3 where X = Cl, Br, I), which demonstrated huge potential in photovoltaics(8-11), also have promising optical gain. Their ultra-stable amplified spontaneous emission at strikingly low thresholds stems from their large absorption coeffcients, ultralow bulk defect densities and slow Auger recombination. Straightforward visible spectral tunability (390-790 nm) is demonstrated. Importantly, in view of their balanced ambipolar charge transport characteristics(8), these materials may show electrically driven lasing.

  • Details
  • Metrics
Type
research article
DOI
10.1038/Nmat3911
Web of Science ID

WOS:000334845600018

Author(s)
Xing, Guichuan
Mathews, Nripan
Lim, Swee Sien
Yantara, Natalia
Liu, Xinfeng
Sabba, Dharani
Gratzel, Michael  
Mhaisalkar, Subodh
Sum, Tze Chien
Date Issued

2014

Publisher

Nature Publishing Group

Published in
Nature Materials
Volume

13

Issue

5

Start page

476

End page

480

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LPI  
Available on Infoscience
May 26, 2014
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/103633
Logo EPFL, École polytechnique fédérale de Lausanne
  • Contact
  • infoscience@epfl.ch

  • Follow us on Facebook
  • Follow us on Instagram
  • Follow us on LinkedIn
  • Follow us on X
  • Follow us on Youtube
AccessibilityLegal noticePrivacy policyCookie settingsEnd User AgreementGet helpFeedback

Infoscience is a service managed and provided by the Library and IT Services of EPFL. © EPFL, tous droits réservés