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Critical fluctuations in the spin-orbit Mott insulator Sr3Ir2O7

Vale, J. G.
•
Boseggia, S.
•
Walker, H. C.
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May 8, 2019
Journal of Physics: Condensed Matter

X-ray magnetic critical scattering measurements and specific heat measurements were performed on the perovskite iridate Sr3Ir2O7. We find that the magnetic interactions close to the Neel temperature T-N = 283.4(2) K are three-dimensional. This contrasts with previous studies which suggest two-dimensional behaviour like Sr2IrO4. Violation of the Harris criterion (d nu > 2) means that weak disorder becomes relevant. This leads a rounding of the antiferromagnetic phase transition at T-N, and modifies the critical exponents relative to the clean system. Specifically, we determine that the critical behaviour of Sr3Ir2O7 is representative of the diluted 3D Ising universality class.

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Vale_2019_J._Phys. _Condens._Matter_31_185803.pdf

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http://purl.org/coar/version/c_970fb48d4fbd8a85

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openaccess

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CC BY

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1.67 MB

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422035fced4bb0254e14d75688a82d14

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