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research article

Hybrid halide perovskite neutron detectors

Andricevic, Pavao  
•
Nafradi, Gabor
•
Kollar, Marton  
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August 30, 2021
Scientific Reports

Interest in fast and easy detection of high-energy radiation (x-, gamma-rays and neutrons) is closely related to numerous practical applications ranging from biomedicine and industry to homeland security issues. In this regard, crystals of hybrid halide perovskite have proven to be excellent detectors of x- and gamma-rays, offering exceptionally high sensitivities in parallel to the ease of design and handling. Here, we demonstrate that by assembling a methylammonium lead tri-bromide perovskite single crystal (CH3NH3PbBr3 SC) with a Gadolinium (Gd) foil, one can very efficiently detect a flux of thermal neutrons. The neutrons absorbed by the Gd foil turn into gamma-rays, which photo-generate charge carriers in the CH3NH3PbBr3 SC. The induced photo-carriers contribute to the electric current, which can easily be measured, providing information on the radiation intensity of thermal neutrons. The dependence on the beam size, bias voltage and the converting distance is investigated. To ensure stable and efficient charge extraction, the perovskite SCs were equipped with carbon electrodes. Furthermore, other types of conversion layers were also tested, including borated polyethylene sheets as well as Gd grains and Gd2O3 pellets directly engulfed into the SCs. Monte Carlo N-Particle (MCNP) radiation transport code calculations quantitatively confirmed the detection mechanism herein proposed.

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Type
research article
DOI
10.1038/s41598-021-95586-3
Web of Science ID

WOS:000693354000034

Author(s)
Andricevic, Pavao  
Nafradi, Gabor
Kollar, Marton  
Nafradi, Balint  
Lilley, Steven
Kinane, Christy
Frajtag, Pavel  
Sienkiewicz, Andrzej  
Pautz, Andreas  
Horvath, Endre  
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Date Issued

2021-08-30

Publisher

Nature Portfolio

Published in
Scientific Reports
Volume

11

Issue

1

Article Number

17159

Subjects

Multidisciplinary Sciences

•

Science & Technology - Other Topics

•

x-ray-detectors

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single-crystals

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gadolinium

•

performance

•

diodes

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

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LRS  
LPMC  
Available on Infoscience
September 25, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/181714
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