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research article

Spiral spin-liquid and the emergence of a vortex-like state in MnSc2S4

Gao, Shang
•
Zaharko, Oksana
•
Tsurkan, Vladimir
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2017
Nature Physics

Spirals and helices are common motifs of long-range order in magnetic solids, and they may also be organized into more complex emergent structures such as magnetic skyrmions and vortices. A new type of spiral state, the spiral spin-liquid, in which spins fluctuate collectively as spirals, has recently been predicted to exist. Here, using neutron scattering techniques, we experimentally prove the existence of a spiral spin-liquid in MnSc2S4 by directly observing the 'spiral surface' a continuous surface of spiral propagation vectors in reciprocal space. We elucidate the multi-step ordering behaviour of the spiral spin liquid, and discover a vortex-like triple-q phase on application of a magnetic field. Our results prove the effectiveness of the J(1)-J(2) Hamiltonian on the diamond lattice as a model for the spiral spin-liquid state in MnSc2S4, and also demonstrate a new way to realize a magnetic vortex lattice through frustrated interactions.

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Type
research article
DOI
10.1038/Nphys3914
Web of Science ID

WOS:000394070700022

Author(s)
Gao, Shang
Zaharko, Oksana
Tsurkan, Vladimir
Su, Yixi
White, Jonathan S.
Tucker, Gregory S.  
Roessli, Bertrand
Bourdarot, Frederic
Sibille, Romain
Chernyshov, Dmitry
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Date Issued

2017

Publisher

Nature Publishing Group

Published in
Nature Physics
Volume

13

Issue

2

Start page

157

End page

161

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
Available on Infoscience
March 27, 2017
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/135914
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