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research article

Nonlinear optical diode effect in a magnetic Weyl semimetal

Tzschaschel, Christian
•
Qiu, Jian-Xiang
•
Gao, Xue-Jian
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April 8, 2024
Nature Communications

Diode effects are of great interest for both fundamental physics and modern technologies. Electrical diode effects (nonreciprocal transport) have been observed in Weyl systems. Optical diode effects arising from the Weyl fermions have been theoretically considered but not probed experimentally. Here, we report the observation of a nonlinear optical diode effect (NODE) in the magnetic Weyl semimetal CeAlSi, where the magnetization introduces a pronounced directionality in the nonlinear optical second-harmonic generation (SHG). We demonstrate a six-fold change of the measured SHG intensity between opposite propagation directions over a bandwidth exceeding 250 meV. Supported by density-functional theory, we establish the linearly dispersive bands emerging from Weyl nodes as the origin of this broadband effect. We further demonstrate current-induced magnetization switching and thus electrical control of the NODE. Our results advance ongoing research to identify novel nonlinear optical/transport phenomena in magnetic topological materials and further opens new pathways for the unidirectional manipulation of light.|Here the authors demonstrate a broadband nonlinear optical diode effect and its electric control in the magnetic Weyl semimetal CeAlSi. Their findings advance ongoing research to identify novel optical phenomena in topological materials.

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Type
research article
DOI
10.1038/s41467-024-47291-8
Web of Science ID

WOS:001198902100031

Author(s)
Tzschaschel, Christian
Qiu, Jian-Xiang
Gao, Xue-Jian
Li, Hou-Chen
Guo, Chunyu  
Yang, Hung-Yu
Zhang, Cheng-Ping
Xie, Ying-Ming
Liu, Yu-Fei
Gao, Anyuan
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Date Issued

2024-04-08

Publisher

Nature Portfolio

Published in
Nature Communications
Volume

15

Issue

1

Article Number

3017

Subjects

Shape Anisotropy

•

Approximation

•

Generation

•

Tool

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
QMAT  
FunderGrant Number

National Science Foundation (NSF)

DE-AC0207CH11358

U.S. Department of Energy (DOE) Office of Science

FA9550-23-1-0040

AFOSR

DMR-2143177

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Available on Infoscience
July 3, 2024
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/208970
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