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research article

Evidence for biquadratic exchange in the quasi-two-dimensional antiferromagnet FePS3

Wildes, A. R.
•
Zhitomirsky, M. E.
•
Ziman, T.
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June 14, 2020
Journal Of Applied Physics

FePS3 is a van der Waals compound with a honeycomb lattice that is a good example of a two-dimensional antiferromagnet with Ising-like anisotropy. Neutron spectroscopy data from FePS3 were previously analyzed using a straightforward Heisenberg Hamiltonian with a single-ion anisotropy. The analysis captured most of the elements of the data; however, some significant discrepancies remained. The discrepancies were most obvious at the Brillouin zone boundaries. The data are subsequently reanalyzed, allowing for unequal exchange between nominally equivalent nearest-neighbors, which resolves the discrepancies. The source of the unequal exchange is attributed to a biquadratic exchange term in the Hamiltonian, which most probably arises from a strong magnetolattice coupling. The new parameters show that there are features consistent with Dirac magnon nodal lines along certain Brillouin zone boundaries.

  • Details
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Type
research article
DOI
10.1063/5.0009114
Web of Science ID

WOS:000541081600002

Author(s)
Wildes, A. R.
Zhitomirsky, M. E.
Ziman, T.
Lancon, D.  
Walker, H. C.
Date Issued

2020-06-14

Publisher

AMER INST PHYSICS

Published in
Journal Of Applied Physics
Volume

127

Issue

22

Article Number

223903

Subjects

Physics, Applied

•

Physics

•

magnetic order

•

transition

•

model

•

mn

•

fe

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
Available on Infoscience
July 4, 2020
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/169835
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