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research article

Direct observation of spin correlations in an artificial triangular lattice Ising spin system with grazing-incidence small-angle neutron scattering

Pip, Petai
•
Glavic, Artur
•
Skjaervo, Sandra Helen
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May 7, 2021
Nanoscale Horizons

The triangular lattice with Ising magnetic moments is an archetypical example of geometric frustration. In the case of dipolar-coupled out-of-plane moments, the geometric frustration results in a disordered classical spin-liquid state at higher temperatures while the system is predicted to transition to an anti-ferromagnetic stripe ground state at low temperatures. In this work we fabricate artificial triangular Ising spin systems without and with uniaxial in-plane compression to tune the nature and temperature of the correlations. We probe the energy scale and nature of magnetic correlations by grazing-incidence small-angle neutron scattering. In particular, we apply a newly-developed empirical structure-factor model to describe the measured short-range correlated spin-liquid state, and find good agreement with theoretical predictions. We demonstrate that grazing-incidence neutron scattering on our high-quality samples, in conjunction with detailed modeling of the scattering using the Distorted Wave Born Approximation, can be used to experimentally quantify the spin-liquid-like correlations in highly-frustrated artificial spin systems.

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Type
research article
DOI
10.1039/d1nh00043h
Web of Science ID

WOS:000648033800001

Author(s)
Pip, Petai
Glavic, Artur
Skjaervo, Sandra Helen
Weber, Anja
Smerald, Andrew  
Zhernenkov, Kirill
Leo, Naemi
Mila, Frederic  
Philippe, Laetitia
Heyderman, Laura J.
Date Issued

2021-05-07

Publisher

ROYAL SOC CHEMISTRY

Published in
Nanoscale Horizons
Volume

6

Issue

6

Start page

474

End page

481

Subjects

Chemistry, Physical

•

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Chemistry

•

Science & Technology - Other Topics

•

Materials Science

•

phase

•

ice

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
CTMC  
Available on Infoscience
May 22, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/178325
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