Repository logo

Infoscience

  • English
  • French
Log In
Logo EPFL, École polytechnique fédérale de Lausanne

Infoscience

  • English
  • French
Log In
  1. Home
  2. Academic and Research Output
  3. Journal articles
  4. Continuous measurements of methane mixing ratios from ice cores
 
research article

Continuous measurements of methane mixing ratios from ice cores

Stowasser, C.
•
Buizert, C.
•
Gkinis, V.
Show more
May 9, 2012
Atmospheric Measurement Techniques

This work presents a new, field-deployable technique for continuous, high-resolution measurements of methane mixing ratios from ice cores. The technique is based on a continuous flow analysis system, where ice core samples cut along the long axis of an ice core are melted continuously. The past atmospheric air contained in the ice is separated from the melt water stream via a system for continuous gas extraction. The extracted gas is dehumidified and then analyzed by a Wavelength Scanned-Cavity Ring Down Spectrometer for methane mixing ratios. We assess the performance of the new measurement technique in terms of precision (±0.8 ppbv,), accuracy (±8 ppbv), temporal (ca. 100 s), and spatial resolution (ca. 5 cm). Using a firn air transport model, we compare the resolution of the measurement technique to the resolution of the atmospheric methane signal as preserved in ice cores in Greenland. We conclude that our measurement technique can resolve all climatically relevant variations as preserved in the ice down to an ice depth of at least 1980 m (66 000 yr before present) in the North Greenland Eemian Ice Drilling ice core. Furthermore, we describe the modifications, which are necessary to make a commercially available spectrometer suitable for continuous methane mixing ratio measurements from ice cores. © Author(s) 2012. CC Attribution 3.0 License.

  • Files
  • Details
  • Metrics
Type
research article
DOI
10.5194/amt-5-999-2012
Web of Science ID

WOS:000304057300007

Author(s)
Stowasser, C.
Buizert, C.
Gkinis, V.
Chappellaz, J.
Schuepbach, S.
Bigler, M.
Fain, X.
Sperlich, P.
Baumgartner, M.
Schilt, A.
Show more
Date Issued

2012-05-09

Publisher

Copernicus GmbH

Published in
Atmospheric Measurement Techniques
Volume

5

Issue

5

Start page

999

End page

1013

Subjects

atmospheric pollution

•

Eemian

•

ice core

•

ice thickness

•

meltwater

•

methane

•

mixing ratio

•

sampling

•

spatial resolution

•

Arctic

•

Greenland

Editorial or Peer reviewed

REVIEWED

Written at

OTHER

EPFL units
SENSE  
Available on Infoscience
November 23, 2022
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/192616
Logo EPFL, École polytechnique fédérale de Lausanne
  • Contact
  • infoscience@epfl.ch

  • Follow us on Facebook
  • Follow us on Instagram
  • Follow us on LinkedIn
  • Follow us on X
  • Follow us on Youtube
AccessibilityLegal noticePrivacy policyCookie settingsEnd User AgreementGet helpFeedback

Infoscience is a service managed and provided by the Library and IT Services of EPFL. © EPFL, tous droits réservés