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  4. Thermal Conductivity of Monolayer Molybdenum Disulfide Obtained from Temperature-Dependent Raman Spectroscopy
 
research article

Thermal Conductivity of Monolayer Molybdenum Disulfide Obtained from Temperature-Dependent Raman Spectroscopy

Yan, Rusen
•
Simpson, Jeffrey R.
•
Bertolazzi, Simone  
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2014
ACS Nano

Atomically thin molybdenum disulfide (MoS2) offers potential for advanced devices and an alternative to graphene due to its unique electronic and optical properties. The temperature-dependent Raman spectra of exfoliated, monolayer MoS2 in the range of 100-320 K are reported and analyzed. The linear temperature coefficients of the in-plane E-2g(1) and the out-of-plane A(1g) modes for both suspended and substrate-supported monolayer MoS2 are measured. These data, when combined with the first-order coefficients from laser power-dependent studies, enable the thermal conductivity to be extracted. The resulting thermal conductivity kappa = (34.5 +/- 4) W/mK at room temperature agrees well with the first-principles lattice dynamics simulations. However, this value is significantly lower than that of graphene. The results from this work provide important input for the design of MoS2-based devices where thermal management is critical.

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Type
research article
DOI
10.1021/nn405826k
Web of Science ID

WOS:000330542900103

Author(s)
Yan, Rusen
Simpson, Jeffrey R.
Bertolazzi, Simone  
Brivio, Jacopo  
Watson, Michael
Wu, Xufei
Kis, Andras  
Luo, Tengfei
Walker, Angela R. Hight
Xing, Huili Grace
Date Issued

2014

Publisher

American Chemical Society

Published in
ACS Nano
Volume

8

Issue

1

Start page

986

End page

993

Subjects

molybdenum disulfide

•

thermal conductivity

•

Raman spectroscopy

•

first-principle lattice dynamics

•

suspended

Editorial or Peer reviewed

REVIEWED

Written at

OTHER

EPFL units
LANES  
Available on Infoscience
March 3, 2014
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/101321
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