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research article

Suppression of ferromagnetic correlations in hole-doped SrCo2As2

Morena, M.
•
van der Spuy, A.
•
Liu, Y.  
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April 1, 2025
Journal Of Physics-materials

We report the growth of high-quality single crystals of hole-doped composition Sr0.95K0.05Co2As2 and present an investigation of its structural, electronic, thermal, and magnetic properties. Our results show that hole doping leads to a substantial suppression of ferromagnetic (FM) correlations present in SrCo2As(2) leading to nearly isotropic magnetic susceptibilities chi(ab,c)(T) of Sr0.95K0.05Co2As2. The presence of FM fluctuations is considered one of the detrimental reasons why SrCo2As2 does not achieve a superconducting ground state despite having a precursor for it in the form of stripe-like antiferromagnetic fluctuations. The suppression of FM fluctuations leads to qualitative similarities between the properties of hole-doped SrCo2As2 and the end member of superconducting 122 iron-arsenide family KFe2As2. Our results also infer the presence of strongly correlated electronic states in Sr0.95K0.05Co2As2. Further, they show that the electronic structure of SrCo2As2 as well as this hole-doped composition is exceptionally unstable in the vicinity of Fermi level E-F for small alterations in the structural parameters and sensitively depends upon the details of simulation.

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Type
research article
DOI
10.1088/2515-7639/adb801
Web of Science ID

WOS:001438542600001

Author(s)
Morena, M.

University of Witwatersrand

van der Spuy, A.

University of Witwatersrand

Liu, Y.  

École Polytechnique Fédérale de Lausanne

Warmbier, R.

University of Witwatersrand

Pandey, Abhishek

University of Witwatersrand

Date Issued

2025-04-01

Publisher

IOP Publishing Ltd

Published in
Journal Of Physics-materials
Volume

8

Issue

2

Article Number

025009

Subjects

SrCo2As2

•

strongly correlated systems

•

magnetic interactions

•

magnetic fluctuations

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LASA  
FunderFunding(s)Grant NumberGrant URL

National Research Foundation - South Africa

SRUG2205098188

Friedel Sellschop fellowship of the University of the Witwatersrand, South Africa

United States Department of Energy (DOE)

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Available on Infoscience
March 18, 2025
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/247967
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