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research article

Low-energy spin dynamics of the s=1/2 kagome system herbertsmithite

Nilsen, G. J.
•
De Vries, M. A.
•
Stewart, J. R.
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2013
Journal of Physics: Condensed Matter

The low-energy (epsilon = (h) over bar < 1 meV), low-temperature (T = 0.05 K) spin dynamics of the s = 1/2 kagome candidate herbertsmithite are probed in the presence of magnetic fields up to 2.5 T. The zero-field spectra reveal a very weak continuum of scattering at T = 10 K and a broad inelastic peak centred at epsilon(max) = 0.2 meV at lower temperatures, T < 1 K. The broad peak is found to be strongly damped, with a liquid-like structure factor implying correlations at length scales up to r = 6 angstrom. The field dependence of the peak appears to follow the Zeeman splitting of s = 1/2 excitations, consistent with the weakly split 'doublets' observed in low-temperature specific heat. A possible explanation of these observations is a short-range correlated state involving defect spins between the kagome planes and moments in the kagome layers.

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Type
research article
DOI
10.1088/0953-8984/25/10/106001
Web of Science ID

WOS:000315195600020

Author(s)
Nilsen, G. J.
•
De Vries, M. A.
•
Stewart, J. R.
•
Harrison, A.
•
Ronnow, Henrik M.  
Date Issued

2013

Publisher

Institute of Physics

Published in
Journal of Physics: Condensed Matter
Volume

25

Issue

10

Article Number

106001

Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
Available on Infoscience
March 28, 2013
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/90687
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