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  4. Theory of optical second-harmonic and sum-frequency scattering from arbitrarily shaped particles
 
research article

Theory of optical second-harmonic and sum-frequency scattering from arbitrarily shaped particles

de Beer, Alex G. F.
•
Roke, Sylvie  
•
Dadap, Jerry I.
2011
Journal Of The Optical Society Of America B-Optical Physics

We present a theoretical framework for the generation and scattering of second-harmonic and sum-frequency light from the surface of particles of arbitrary shape in the limit of low index of refraction contrast. For homogeneous and isotropic surfaces, light scattering can be described by a finite set of scattering functions. Selection rules regarding these scattering functions are presented. We also find that the scattering functions associated with achiral and chiral surfaces are directly related to the bulk and surface linear optical form factors, respectively. Finally, we derive explicit expressions for particles of ellipsoidal shape, for which we calculate angular scattering patterns as a function of particle orientation and for ensembles of particles. (C) 2011 Optical Society of America

  • Details
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Type
research article
DOI
10.1364/JOSAB.28.001374
Web of Science ID

WOS:000291314600003

Author(s)
de Beer, Alex G. F.
Roke, Sylvie  
Dadap, Jerry I.
Date Issued

2011

Published in
Journal Of The Optical Society Of America B-Optical Physics
Volume

28

Start page

1374

End page

1384

Subjects

Centrosymmetric Material

•

Colloidal Particles

•

Spherical-Particles

•

Rayleigh-Scattering

•

Light-Scattering

•

Generation

•

Surface

•

Spectroscopy

•

Nanoparticles

•

Nanocrystals

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LBP  
Available on Infoscience
December 16, 2011
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/74018
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