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research article

Atom-surface van der Waals potentials of topological insulators and semimetals from scattering measurements

Tamtoegl, Anton
•
Ruckhofer, Adrian
•
Campi, Davide  
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April 7, 2021
Physical Chemistry Chemical Physics

The phenomenology of resonant scattering has been known since the earliest experiments upon scattering of atomic beams from surfaces and is a means of obtaining experimental information about the fundamentals of weak adsorption systems in the van der Waals regime. We provide an overview of the experimental approach based on new experimental data for the He-Sb2Te3(111) system, followed by a comparative overview and perspective of recent results for topological semimetal and insulator surfaces. Moreover, we shortly discuss the perspectives of calculating helium-surface interaction potentials from ab initio calculations. Our perspective demonstrates that atom-surface scattering provides direct experimental information about the atom-surface interaction in the weak physisorption regime and can also be used to determine the lifetime and mean free path of the trapped atom. We further discuss the effects of elastic and inelastic scattering on the linewidth and lifetime of the trapped He atom with an outlook on future developments and applications.

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Type
research article
DOI
10.1039/d0cp05388k
Web of Science ID

WOS:000646815600006

Author(s)
Tamtoegl, Anton
Ruckhofer, Adrian
Campi, Davide  
Allison, William
Ernst, Wolfgang E.
Date Issued

2021-04-07

Published in
Physical Chemistry Chemical Physics
Volume

23

Issue

13

Start page

7637

End page

7652

Subjects

Chemistry, Physical

•

Physics, Atomic, Molecular & Chemical

•

Chemistry

•

Physics

•

selective-adsorption resonances

•

density-functional theory

•

single dirac cone

•

he atoms

•

electronic corrugation

•

elastic-scattering

•

band-structure

•

gas atoms

•

ab-initio

•

helium

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
THEOS  
Available on Infoscience
June 5, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/178563
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