Understanding unconventional magnetic order in a candidate axion insulator by resonant elastic x-ray scattering
Magnetic topological insulators and semimetals are a class of crystalline solids whose properties are strongly influenced by the coupling between non-trivial electronic topology and magnetic spin configurations. Such materials can host exotic electromagnetic responses. Among these are topological insulators with certain types of antiferromagnetic order which are predicted to realize axion electrodynamics. Here we investigate the highly unusual helimagnetic phases recently reported in EuIn2As2, which has been identified as a candidate for an axion insulator. Using resonant elastic x-ray scattering we show that the two types of magnetic order observed in EuIn2As2 are spatially uniform phases with commensurate chiral magnetic structures, ruling out a possible phase-separation scenario, and we propose that entropy associated with low energy spin fluctuations plays a significant role in driving the phase transition between them. Our results establish that the magnetic order in EuIn2As2 satisfies the symmetry requirements for an axion insulator. EuIn2As2 is a candidate as an axion insulator, a material that can host axion-like quasi-particles, in direct analogy with the axion proposed in particle physics to resolve the so called "strong CP problem". Here Soh et al., perform resonant elastic X-Ray scattering on EuIn2As2 and show that the magnetic order consists of commensurate chiral magnetic structures, satisfying the symmetry requirements for EuIn2As2 to be an axion insulator.'
document.pdf
Publisher's version
openaccess
CC BY
1.39 MB
Adobe PDF
c41359108d4acb57ebcf03268d972b7b