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  4. Heralded Spectroscopy: a new single-particle probe for nanocrystal photophysics
 
conference paper

Heralded Spectroscopy: a new single-particle probe for nanocrystal photophysics

Lubin, Gur
•
Tenne, Ron
•
Ulku, Arin Can  
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January 1, 2023
Single Molecule Spectroscopy And Superresolution Imaging Xvi
Conference on Single Molecule Spectroscopy and Superresolution Imaging XVI

Semiconductor nanocrystals feature multiply-excited states that display intriguing physics and significantly impact nanocrystal-based technologies. Fluorescence supplies a natural probe to investigate these states. Still, direct observation of multiexciton fluorescence has proved elusive to existing spectroscopy techniques. Heralded Spectroscopy is a new tool based on a breakthrough single-particle, single-photon, sub-nanosecond spectrometer that utilizes temporal photon correlations to isolate multiexciton emission. This proceedings paper introduces Heralded Spectroscopy and reviews some of the novel insights it uncovered into exciton-exciton interactions within single nanocrystals. These include weak exciton-exciton interactions and their correlation with quantum confinement, biexciton spectral diffusion, multiple biexciton species and biexciton emission polarization.

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Type
conference paper
DOI
10.1117/12.2650463
Web of Science ID

WOS:001011711100002

Author(s)
Lubin, Gur
•
Tenne, Ron
•
Ulku, Arin Can  
•
Antolovic, Ivan Michel  
•
Burri, Samuel  
•
Karg, Sean
•
Yallapragada, Venkata Jayasurya
•
Yaniv, Gili
•
Kazes, Miri
•
Amgar, Daniel
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Date Issued

2023-01-01

Publisher

SPIE-INT SOC OPTICAL ENGINEERING

Publisher place

Bellingham

Published in
Single Molecule Spectroscopy And Superresolution Imaging Xvi
ISBN of the book

978-1-5106-5877-6

978-1-5106-5878-3

Series title/Series vol.

Progress in Biomedical Optics and Imaging

Volume

12386

Start page

1238603

Subjects

Computer Science, Interdisciplinary Applications

•

Optics

•

Computer Science

•

quantum dots

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multiexcitons

•

biexciton binding energy

•

single-particle spectroscopy

•

spad arrays

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perovskite nanocrystals

Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
AQUA  
Event nameEvent placeEvent date
Conference on Single Molecule Spectroscopy and Superresolution Imaging XVI

San Francisco, CA

Jan 28-29, 2023

Available on Infoscience
July 31, 2023
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/199526
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