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research article

Characterization of two electronic subsystems in cuprates through optical conductivity

Kumar, C. M. N.
•
Akrap, A.
•
Homes, C. C.
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April 27, 2023
Physical Review B

Understanding the physical properties of unconventional superconductors as well as of other correlated materials presents a formidable challenge. Their unusual evolution with doping, frequency, and temperature has frequently led to non-Fermi-liquid (non-FL) interpretations. Optical conductivity is a major challenge in this context. Here, the optical spectra of two archetypal cuprates, underdoped HgBa2CuO4+delta; and optimally doped Bi2Sr2CaCu2O8+delta, are interpreted based on the standard Fermi-liquid (FL) paradigm. At both dopings, perfect frequency-temperature FL scaling is found to be modified by the presence of a second, gapped electronic subsystem. This non-FL component emerges as a well-defined mid-infrared spectral feature after the FL contribution, determined independently by transport, is subtracted. Temperature, frequency, and doping evolution of the MIR feature identify a gapped rather than dissipative response. In contrast, the dissipative response is found to be relevant for pnictides and ruthenates. Such an unbiased FL/non-FL separation is extended across the cuprate phase diagram, capturing all the key features of the normal state and providing a natural explanation why the superfluid density is attenuated on the overdoped side. Thus, we obtain a unified interpretation of optical responses and transport measurements in all analyzed physical regimes and all analyzed compounds.

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Type
research article
DOI
10.1103/PhysRevB.107.144515
Web of Science ID

WOS:000985670600004

Author(s)
Kumar, C. M. N.
Akrap, A.
Homes, C. C.
Martino, E.  
Klebel-Knobloch, B.
Tabis, W.
Barisic, O. S.
Sunko, D. K.
Barisic, N.
Date Issued

2023-04-27

Published in
Physical Review B
Volume

107

Issue

14

Article Number

144515

Subjects

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Materials Science

•

Physics

•

fermi-surface

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temperature-dependence

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band-structure

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superconductivity

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energy

•

state

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phase

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

Available on Infoscience
June 5, 2023
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/198104
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