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  4. Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields
 
research article

Ultrafast Transverse Modulation of Free Electrons by Interaction with Shaped Optical Fields

Madan, Ivan  
•
Leccese, Veronica  
•
Mazur, Adam
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September 27, 2022
Acs Photonics

Spatiotemporal electron-beam shaping is a bold frontier of electron microscopy. Over the past decade, shaping methods evolved from static phase plates to low-speed electrostatic and magnetostatic displays. Recently, a swift change of paradigm utilizing light to control free electrons has emerged. Here, we experimentally demonstrate arbitrary transverse modulation of electron beams without complicated electron-optics elements or material nanostructures, but rather using shaped light beams. On-demand spatial modulation of electron wavepackets is obtained via inelastic interaction with transversely shaped ultrafast light fields controlled by an external spatial light modulator. We illustrate this method for the cases of Hermite-Gaussian and Laguerre-Gaussian modulation and discuss their use in enhancing microscope sensitivity. Our approach dramatically widens the range of patterns that can be imprinted on the electron profile and greatly facilitates tailored electron-beam shaping.

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Type
research article
DOI
10.1021/acsphotonics.2c00850
Web of Science ID

WOS:000863580800001

Author(s)
Madan, Ivan  
•
Leccese, Veronica  
•
Mazur, Adam
•
Barantani, Francesco  
•
LaGrange, Thomas  
•
Sapozhnik, Alexey  
•
Tengdin, Phoebe M.
•
Gargiulo, Simone  
•
Rotunno, Enzo
•
Olaya, Jean-Christophe
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Date Issued

2022-09-27

Publisher

AMER CHEMICAL SOC

Published in
Acs Photonics
Volume

9

Issue

10

Start page

3215

End page

3224

Subjects

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Optics

•

Physics, Applied

•

Physics, Condensed Matter

•

Science & Technology - Other Topics

•

Materials Science

•

Physics

•

electron-beam shaping electron-photon interaction

•

pinem

•

ultrafast transmission electron microscopy

•

spatial light modulator

•

phase plates

•

microscopy

•

beams

•

spectroscopy

•

diffraction

•

generation

•

wave

•

weak

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LUMES  
Available on Infoscience
October 24, 2022
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/191629
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