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research article

Nonequilibrium quasistationary spin disordered state in ?-RuCl3

Versteeg, R. B.
•
Chiocchetta, A.
•
Sekiguchi, F.
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June 30, 2022
Physical Review B

We photoexcite high-energy holon-doublon pairs as a way to alter the magnetic free energy landscape and resulting phase diagram of the frustrated honeycomb magnet ??-RuCl3. The pair recombination through multimagnon emission is tracked through the time evolution of the magnetooptical response originating from ??-RuCl3???s competing zigzag spin-ordered ground state. A small holon-doublon density suffices to reach a spin-disordered state. The phase transition is described within a dynamical Ginzburg-Landau framework, corroborating the quasistationary nature of the transient phase. Our work suggests a new route to reach a nontrivial spin-disordered state in Kitaev-like magnets.

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Type
research article
DOI
10.1103/PhysRevB.105.224428
Web of Science ID

WOS:000823037600004

Author(s)
Versteeg, R. B.
Chiocchetta, A.
Sekiguchi, F.
Sahasrabudhe, A.
Wagner, J.
Aldea, A. I. R.
Budzinauskas, K.
Wang, Zhe  
Tsurkan, V.
Loidl, A.
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Date Issued

2022-06-30

Publisher

AMER PHYSICAL SOC

Published in
Physical Review B
Volume

105

Issue

22

Article Number

224428

Subjects

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Materials Science

•

Physics

•

quantum

•

ferroelectricity

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
PRST  
Available on Infoscience
August 1, 2022
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/189673
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