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  4. Ultrafast Momentum-Resolved Free-Electron Probing of Optically Pumped Plasmon Thermal Dynamics
 
research article

Ultrafast Momentum-Resolved Free-Electron Probing of Optically Pumped Plasmon Thermal Dynamics

Mkhitaryan, Vahagn
•
Dias, Eduardo J. C.
•
Carbone, Fabrizio  
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February 17, 2021
Acs Photonics

Current advances in ultrafast electron microscopy make it possible to combine optical pumping of a nanostructure and electron beam probing with sub-Angstrom and femtosecond spatiotemporal resolution. We present a theory predicting that this technique can reveal a rich out-of-equilibrium dynamics of plasmon excitations in graphene and graphite samples. In a disruptive departure from the traditional probing of nanoscale excitations based on the identification of spectral features in the transmitted electrons, we show that the measurement of angle-resolved, energy-integrated inelastic electron scattering can trace the temporal evolution of plasmons in these structures and provide momentum-resolved mode identification, thus avoiding the need for highly monochromatic electron beams and the use of electron spectrometers. This previously unexplored approach to study the ultrafast dynamics of optical excitations can be of interest to understand and manipulate polaritons in 2D semiconductors and other materials exhibiting a strong thermo-optical response.

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Type
research article
DOI
10.1021/acsphotonics.0c01758
Web of Science ID

WOS:000621063700029

Author(s)
Mkhitaryan, Vahagn
Dias, Eduardo J. C.
Carbone, Fabrizio  
Garcia de Abajo, F. Javier
Date Issued

2021-02-17

Publisher

AMER CHEMICAL SOC

Published in
Acs Photonics
Volume

8

Issue

2

Start page

614

End page

624

Subjects

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Optics

•

Physics, Applied

•

Physics, Condensed Matter

•

Science & Technology - Other Topics

•

Materials Science

•

Physics

•

ultrafast plasmon dynamics

•

ultrafast electron microscopy

•

graphene plasmons

•

thermo-optical response

•

eels

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LUMES  
Available on Infoscience
April 10, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/177159
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