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  4. Light-Induced Renormalization of the Dirac Quasiparticles in the Nodal-Line Semimetal ZrSiSe
 
research article

Light-Induced Renormalization of the Dirac Quasiparticles in the Nodal-Line Semimetal ZrSiSe

Gatti, G.  
•
Crepaldi, A.  
•
Puppin, M.  
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August 12, 2020
Physical Review Letters

In nodal-line semimetals, linearly dispersing states form Dirac loops in the reciprocal space with a high degree of electron-hole symmetry and a reduced density of states near the Fermi level. The result is reduced electronic screening and enhanced correlations between Dirac quasiparticles. Here we investigate the electronic structure of ZrSiSe, by combining time- and angle-resolved photoelectron spectroscopy with ab initio density functional theory (DFT) complemented by an extended Hubbard model (DFT + U + V) and by time-dependent DFT + U + V. We show that electronic correlations are reduced on an ultrashort timescale by optical excitation of high-energy electrons-hole pairs, which transiently screen the Coulomb interaction. Our findings demonstrate an all-optical method for engineering the band structure of a quantum material.

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Type
research article
DOI
10.1103/PhysRevLett.125.076401
Web of Science ID

WOS:000558600800008

Author(s)
Gatti, G.  
Crepaldi, A.  
Puppin, M.  
Tancogne-Dejean, N.
Xian, L.
De Giovannini, U.
Roth, S.
Polishchuk, S.  
Bugnon, Ph  
Magrez, A.  
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Date Issued

2020-08-12

Published in
Physical Review Letters
Volume

125

Issue

7

Article Number

076401

Subjects

Physics, Multidisciplinary

•

Physics

•

1st-principles

•

dynamics

•

spin

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSU  
LSE  
LNNME  
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Available on Infoscience
August 27, 2020
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/171167
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