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review article

Review on Recent Progress of All-Inorganic Metal Halide Perovskites and Solar Cells

Xiang, Wanchun
•
Tress, Wolfgang  
September 3, 2019
Advanced Materials

All-inorganic perovskites are considered to be one of the most appealing research hotspots in the field of perovskite photovoltaics in the past 3 years due to their superior thermal stability compared to their organic-inorganic hybrid counterparts. The power-conversion efficiency has reached 17.06% and the number of important publications is ever increasing. Here, the progress of inorganic perovskites is systematically highlighted, covering materials design, preparation of high-quality perovskite films, and avoidance of phase instabilities. Inorganic perovskites, nanocrystals, quantum dots, and lead-free compounds are discussed and the corresponding device performances are reviewed, which have been realized on both rigid and flexible substrates. Methods for stabilization of the cubic phase of low-bandgap inorganic perovskites are emphasized, which is a prerequisite for highly efficient and stable solar cells. In addition, energy loss mechanisms both in the bulk of the perovskite and at the interfaces of perovskite and charge selective layers are unraveled. Reported approaches to reduce these charge-carrier recombination losses are summarized and complemented by methods proposed from our side. Finally, the potential of inorganic perovskites as stable absorbers is assessed, which opens up new perspectives toward the commercialization of inorganic perovskite solar cells.

  • Details
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Type
review article
DOI
10.1002/adma.201902851
Web of Science ID

WOS:000484855300001

Author(s)
Xiang, Wanchun
Tress, Wolfgang  
Date Issued

2019-09-03

Publisher

Wiley-V C H Verlag Gmbh

Published in
Advanced Materials
Article Number

1902851

Subjects

Chemistry, Multidisciplinary

•

Chemistry, Physical

•

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Chemistry

•

Science & Technology - Other Topics

•

Materials Science

•

Physics

•

energy loss

•

inorganic perovskites

•

power conversion efficiency

•

solar cells

•

stability

•

highly efficient

•

thin-films

•

thermal-stability

•

cspbi2br

•

phase

•

nanocrystals

•

performance

•

alpha-cspbi3

•

fabrication

•

cs2agbibr6

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LPI  
Available on Infoscience
September 25, 2019
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/161512
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