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research article

Upgrade of a low-temperature scanning tunneling microscope for electron-spin resonance

Natterer, Fabian D.  
•
Patthey, Francois  
•
Bilgeri, Tobias  
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January 1, 2019
Review Of Scientific Instruments

Electron spin resonance with a scanning tunneling microscope (ESR-STM) combines the high energy resolution of spin resonance spectroscopy with the atomic scale control and spatial resolution of STM. Here we describe the upgrade of a helium-3 STM with a 2D vector-field magnet (B-z = 8.0 T, B-x = 0.8 T) to an ESR-STM. The system is capable of delivering radio frequency (RF) power to the tunnel junction at frequencies up to 30 GHz. We demonstrate magnetic field-sweep ESR for the model system TiH/MgO/Ag(100) and find a magnetic moment of (1.004 +/- 0.001)mu(B). Our upgrade enables to toggle between a DC mode, where the STM is operated with the regular control electronics, and an ultrafast-pulsed mode that uses an arbitrary waveform generator for pump-probe spectroscopy or reading of spin-states. Both modes allow for simultaneous radiofrequency excitation, which we add via a resistive pick-off tee to the bias voltage path. The RF cabling from room temperature to the 350 mK stage has an average attenuation of 18 dB between 5 and 25 GHz. The cable segment between the 350 mK stage and the STM tip presently attenuates an additional 34(-3)(+5) dB from 10 to 26 GHz and 38(-2)(+3) dB between 20 and 30 GHz. We discuss our transmission losses and indicate ways to reduce this attenuation. We finally demonstrate how to synchronize the arrival times of RF and DC pulses coming from different paths to the STM junction, a prerequisite for future pulsed ESR experiments. Published under license by AIP Publishing.

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Type
research article
DOI
10.1063/1.5065384
Web of Science ID

WOS:000457411800029

Author(s)
Natterer, Fabian D.  
Patthey, Francois  
Bilgeri, Tobias  
Forrester, Patrick R.
Weiss, Nicolas  
Brune, Harald  
Date Issued

2019-01-01

Publisher

AMER INST PHYSICS

Published in
Review Of Scientific Instruments
Volume

90

Issue

1

Article Number

013706

Subjects

Instruments & Instrumentation

•

Physics, Applied

•

Instruments & Instrumentation

•

Physics

•

spectroscopy

•

atoms

•

limit

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LNS  
Available on Infoscience
February 20, 2019
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/154601
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