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research article

Active microrheology in corrugated channels

Puertas, Antonio M.
•
Malgaretti, Paolo
•
Pagonabarraga, Ignacio
November 7, 2018
Journal Of Chemical Physics

We analyze the dynamics of a tracer particle embedded in a bath of hard spheres confined in a channel of varying section. By means of Brownian dynamics simulations, we apply a constant force on the tracer particle and discuss the dependence of its mobility on the relative magnitude of the external force with respect to the entropic force induced by the confinement. A simple theoretical one-dimensional model is also derived, where the contribution from particle-particle and particle-wall interactions is taken from simulations with no external force. Our results show that the mobility of the tracer is strongly affected by the confinement. The tracer velocity in the force direction has a maximum close to the neck of the channel, in agreement with the theory for small forces. Upon increasing the external force, the tracer is effectively confined to the central part of the channel and the velocity modulation decreases, which cannot be reproduced by the theory. This deviation marks the regime of validity of linear response. Surprisingly, when the channel section is not constant, the effective friction coefficient is reduced as compared to the case of a plane channel. The transversal velocity, which cannot be studied with our model, follows qualitatively the derivative of the channel section, in agreement with previous theoretical calculations for the tracer diffusivity in equilibrium. Published by AIP Publishing.

  • Details
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Type
research article
DOI
10.1063/1.5048343
Web of Science ID

WOS:000449558000051

Author(s)
Puertas, Antonio M.
•
Malgaretti, Paolo
•
Pagonabarraga, Ignacio
Date Issued

2018-11-07

Published in
Journal Of Chemical Physics
Volume

149

Issue

17

Article Number

174908

Subjects

Chemistry, Physical

•

Physics, Atomic, Molecular & Chemical

•

Chemistry

•

Physics

•

energy

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
SB  
Available on Infoscience
December 13, 2018
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/152498
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