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research article

Retention of iodine in yttria stabilized zirconia

Pouchon, Manuel A.  
•
Döbeli, Max
•
Degueldre, Claude
1999
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms

The diffusion behavior of iodine in yttria stabilized zirconia (YSZ) was investigated as a function of the temperature. Iodine implantation was performed in this cubic solid solution by irradiating material samples with 1 MeV iodine ions. The distribution of iodine was evaluated by using TRIM computer calculation and measured by Rutherford backscattering spectrometry (RBS) using 5 MeV 4He particle. The iodine profile was quantified after successive temperature steps. At each step the maximum temperature was held for 2 h. It was found, that the iodine profile remained unchanged up to 1373 K. At 1573 K iodine diffused significantly. The iodine profile was measurable up to 1773 K. Even at this high temperature a significant iodine retention is observed. The diffusion coefficient of iodine (3.5 ± 1.4 × 10−15 cm2 s−1) is of the same order as the temperature extrapolated data of iodine in monoclinic/tetragonal zirconia.

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Type
research article
DOI
10.1016/S0168-583X(98)00885-4
Author(s)
Pouchon, Manuel A.  
Döbeli, Max
Degueldre, Claude
Date Issued

1999

Publisher

Elsevier

Published in
Nuclear Instruments and Methods in Physics Research Section B: Beam Interactions with Materials and Atoms
Volume

148

Issue

1-4

Start page

783

End page

786

Subjects

Nuclear fuel

•

Yttria stabilized zirconia

•

YSZ

•

Iodine

•

Retention

•

Diffusion

Editorial or Peer reviewed

REVIEWED

Written at

OTHER

EPFL units
LNM_PSI  
Available on Infoscience
April 14, 2015
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/113315
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