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research article

Nonlinear optical scattering: The concept of effective susceptibility

Roke, S.  
•
Bonn, M.
•
Petukhov, A. V.
2004
Physical Review B

We present a general theoretical method for deriving effective susceptibilities for (non)linear optical scattering processes of arbitrary order using the reciprocity principle. This method allows us to formulate a generalized treatment of nonlinear optical scattering and deduce selection rules independent of the precise mechanism of light-matter interaction. We particularize this approach to second-order sum frequency scattering from an inhomogeneous medium and consider the limiting cases of small particle scattering, refractive index matched (Rayleigh-Gans-Debye) scattering, small refractive index contrast (Wentzel-Kramers-Brillouin) scattering and correlated scattering. We compare the derived expressions to experimental results of sum frequency scattering from monodisperse particles in suspension with varying sizes.

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Type
research article
DOI
10.1103/PhysRevB.70.115106
Scopus ID

2-s2.0-19744381749

Author(s)
Roke, S.  
Bonn, M.
Petukhov, A. V.
Date Issued

2004

Published in
Physical Review B
Volume

70

Issue

11

Start page

115106

End page

1

Editorial or Peer reviewed

REVIEWED

Written at

OTHER

EPFL units
LBP  
Available on Infoscience
February 8, 2013
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/88718
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