Direct comparison of phase-sensitive vibrational sum frequency generation with maximum entropy method: Case study of water

We present a direct comparison of phase sensitive sum-frequency generation experiments with phase reconstruction obtained by the maximum entropy method. We show that both methods lead to the same complex spectrum. Furthermore, we discuss the strengths and weaknesses of each of these methods, analyzing possible sources of experimental and analytical errors. A simulation program for maximum entropy phase reconstruction is available at: http://lbp.epfl.ch/.


Published in:
Journal Of Chemical Physics, 135, 22, 224701
Year:
2011
ISSN:
00219606
Keywords:
Laboratories:




 Record created 2012-06-25, last modified 2018-03-17


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