Interfacial Photoreduction of Supercritical CO2 by an Aqueous Catalyst

Not just a solvent anymore: CO2 reduction under supercritical conditions was achieved in a biphasic water–supercritical CO2 system using an aqueous soluble catalyst (see picture). The introduction of such an interface provides a suitable reaction medium where adsorption, CO2 binding, and protonation of intermediates are intimately linked.


Published in:
Angewandte Chemie-International Edition, 50, 32, 7391-7394
Year:
2011
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 Record created 2011-12-16, last modified 2018-03-17

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