Repository logo

Infoscience

  • English
  • French
Log In
Logo EPFL, École polytechnique fédérale de Lausanne

Infoscience

  • English
  • French
Log In
  1. Home
  2. Academic and Research Output
  3. Journal articles
  4. β-Molybdenum nitride: synthesis mechanism and catalytic response in the gas phase hydrogenation of p-chloronitrobenzene
 
research article

β-Molybdenum nitride: synthesis mechanism and catalytic response in the gas phase hydrogenation of p-chloronitrobenzene

Cardenas-Lizana, Fernando
•
Gomez-Quero, Santiago
•
Perret, Noemie
Show more
2011
Catalysis Science & Technology

A temperature programmed treatment of MoO3 in flowing N-2 + H-2 has been employed to prepare beta-phase molybdenum nitride (beta-Mo2N) which has been used to promote, for the first time, the catalytic hydrogenation of p-chloronitrobenzene. The reduction/nitridation synthesis steps have been monitored in situ and the starting oxide, reaction intermediates and nitride product have been identified and characterized by powder X-ray diffraction (XRD), diffuse reflectance UV-Vis (DRS UV-Vis), elemental analysis, scanning electron microscopy (SEM) and BET/pore volume measurements. Our results demonstrate that MoO3 -> beta-Mo2N is a kinetically controlled process where an initial reduction stage generates (sequentially) MoO2 and Mo as reaction intermediates with a subsequent incorporation of N to produce beta-Mo2N. SEM analysis has established that the transformation is non-topotactic with a disruption to the platelet morphology that characterizes MoO3 and an increase in BET area (from 1 m(2) g(-1) to 17 m(2) g(-1)). Moreover, temperature programmed desorption measurements have revealed a significant hydrogen uptake (0.71 mu mol m(-2)) on beta-Mo2N. This has been exploited in the hydrogenation of p-chloronitrobenzene where p-chloroaniline was generated as the sole product with an associated rate constant (k = 2.0 min(-1)) that is higher than values recorded for supported transition metals. Our study establishes the reaction mechanism involved in the synthesis of beta-Mo2N and demonstrates its viability to promote selective -NO2 group reduction as an alternative sustainable, high throughput route to commercially important haloamines.

  • Details
  • Metrics
Type
research article
DOI
10.1039/c0cy00011f
Web of Science ID

WOS:000294016200012

Author(s)
Cardenas-Lizana, Fernando
Gomez-Quero, Santiago
Perret, Noemie
Kiwi-Minsker, Lioubov  
Keane, Mark A.
Date Issued

2011

Published in
Catalysis Science & Technology
Volume

1

Issue

5

Start page

794

End page

801

Subjects

Temperature-Programmed Desorption

•

In-Situ Xas

•

Surface-Area

•

Carbazole Hydrodenitrogenation

•

Selective Hydrogenation

•

Carbide Catalysts

•

Hydrodesulfurization Catalyst

•

Unsupported Powders

•

Ammonia-Synthesis

•

Metal Carbides

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LGRC  
Available on Infoscience
December 16, 2011
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/73714
Logo EPFL, École polytechnique fédérale de Lausanne
  • Contact
  • infoscience@epfl.ch

  • Follow us on Facebook
  • Follow us on Instagram
  • Follow us on LinkedIn
  • Follow us on X
  • Follow us on Youtube
AccessibilityLegal noticePrivacy policyCookie settingsEnd User AgreementGet helpFeedback

Infoscience is a service managed and provided by the Library and IT Services of EPFL. © EPFL, tous droits réservés