Long-term trends of primary and secondary pollutant concentrations in Switzerland and their response to emission controls and economic changes
A de-trending technique was developed for short-term and annual variations to identify long-term trends in primary and secondary pollutants. With this approach, seasonal and annual variations are removed using a mean year; the residual meteorol. short-term variation is removed using a multiple linear regression model. This method was used to de-trend O3, NOx, volatile org. compd. (VOC) and CO concns. in Switzerland. Primary pollutants (NOx, VOC, CO) at urban and suburban stations exhibited a downward trend over the last decade which correlates well with redns. in estd. Swiss emissions. Despite large decreases achieved in precursor emissions, summer peak O3 concns. did not show any statistically significant trend over the last decade. Applying this method to O3 concns. measured at the Jungfraujoch (3580 m above sea level) also showed no trend over the last 10 yr. De-trended summer O3 correlated well with European Union gross national product and industrial prodn. growth rates. These results suggested that if substantial redns. in summer peak O3 in Switzerland are desired, emissions redn. strategies must be part of control programs involving a much larger region.
2001
35
8
1351
1363
Copyright 2003 ACS
CAPLUS
AN 2001:110382
CAN 134:284861
59-2
Air Pollution and Industrial Hygiene
53
Swiss Federal Institute of Technology,Lausanne,Switz. FIELD URL:
Journal
AENVEQ
written in English.
Air pollution (de-trending method to assess effect of emission controls and economic changes on long-term trends of primary and secondary air pollutants in Switzerland); Volatile organic compounds Role: POL (Pollutant), OCCU (Occurrence) (de-trending method to assess effect of emission controls and economic changes on long-term trends of primary and secondary air pollutants in Switzerland); Simulation and Modeling (meteorol. conditions; de-trending method to assess effect of emission controls and economic changes on long-term trends of primary and secondary air pollutants in Switzerland); Air pollution (photochem.; de-trending method to assess effect of emission controls and economic changes on long-term trends of primary and secondary air pollutants in Switzerland)
Altshuler, S; Journal of the Air and Waste Management Association 1995, 45, 967|Baltensperger, U; Journal of Geophysical Research 1997, 102, 19707|Bronimann, S; Atmospheric Environment 1997, 31, 1127|Clappier, A; European project COST 615-CITAIR, http://dgrwww.epfl.ch/PAS/MOD/study/cost/ 1997|Eidgenossische Komission fur Lufthygiene; Ozone in der Schweiz 1993|Eskridge, R; Bulletin of the American Meteorological Society 1997, 78, 1473|Flaum, J; Journal of the Air and Waste Management Association 1996, 46, 35|Gardner, M; Atmospheric Environment 1999, 34, 171|Graf-Jaccotet, M; Environmetrics 1998, 9, 393|Kahn, M; A Report for the Georgia Department of Natural Resources 2000|Kuebler, J; Atmospheric Environment 1996, 30, 951|Lau, K; Bulletin of the American Meteorological Society 1995, 76, 239|Lugauer, M; Tellus 1998, 50B, 76|Milanchus, M; Presentation at the Air and Waste Management Association's 90th Annual Meeting 1997|Neu, U; Boundary-Layer Meteorology 1994, 69, 221|Perego, S; Research Report for the Canton Obwald, http://dgrwww.epfl.ch/PAS/MOD/obwald 1999|Rao, S; Journal of the Air and Waste Management Association 1994, 44, 1089|SAEFL; Emissions Polluantes dues a l'Activite Humaine en Suisse de 1900 a 2010 1995|SAEFL; NABEL 1998|Stohl, A; Atmospheric Environment 2000, 34, 1323|Swiss Federal Office of Energy; Statistique globale suisse de l'energie 1997 1998|Swiss Federal Office of Energy; Apercu de la consommation d'energie en suisse au cours de l'annee 1998 1999|Thomas, J; Georgia Undergraduate Research Report 2000|Venables, W; Modern Applied Statistics with S-PLUS 1998|Wilks, D; International Geophysics Series 1995, 59|Zanis, P; Atmospheric Environment 1999, 33, 3777|Zurbenko, I; International Statistical Review 1991, 59, 163
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