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research article

A vacuum flash-assisted solution process for high-efficiency large-area perovskite solar cells

Li, Xiong  
•
Bi, Dongqin  
•
Yi, Chenyi  
Show more
2016
Science

Metal halide perovskite solar cells (PSCs) currently attract enormous research interest because of their high solar-to-electric power conversion efficiency (PCE) and low fabrication costs, but their practical development is hampered by difficulties in achieving high performance with large-size devices. We devised a simple vacuum flash-assisted solution processing method to obtain shiny, smooth, crystalline perovskite films of high electronic quality over large areas. This enabled us to fabricate solar cells with an aperture area exceeding 1 square centimeter, a maximum efficiency of 20.5%, and a certified PCE of 19.6%. By contrast, the best certified PCE to date is 15.6% for PSCs of similar size. We demonstrate that the reproducibility of the method is excellent and that the cells show virtually no hysteresis. Our approach enables the realization of highly efficient large-area PSCs for practical deployment.

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Type
research article
DOI
10.1126/science.aaf8060
Web of Science ID

WOS:000378816200034

Author(s)
Li, Xiong  
Bi, Dongqin  
Yi, Chenyi  
Decoppet, Jean-David  
Luo, Jingshan  
Zakeeruddin, Shaik Mohammed  
Hagfeldt, Anders
Gratzel, Michael  
Date Issued

2016

Publisher

American Association for the Advancement of Science

Published in
Science
Volume

353

Issue

6294

Start page

58

End page

62

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LPI  
Available on Infoscience
October 18, 2016
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/129919
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