Probing strongly hybridized nuclear-electronic states in a model quantum ferromagnet
We present direct local-probe evidence for strongly hybridized nuclear-electronic spin states of an Ising ferromagnet LiHoF4 in a transverse magnetic field. The nuclear-electronic states are addressed via a magnetic resonance in the GHz frequency range using coplanar resonators and a vector network analyzer. The magnetic resonance spectrum is successfully traced over the entire field-temperature phase diagram, which is remarkably well reproduced by mean-field calculations. Our method can be directly applied to a broad class of materials containing rare-earth ions for probing the substantially mixed nature of the nuclear and electronic moments.
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Kovacevic, I., Babkevich, P., Jeong, M., Piatek, J. O., Boero, G., & Rønnow, H. M. (2016). Probing strongly hybridized nuclear-electronic states in a model quantum ferromagnet. Physical Review B, 94(21), Article 214433. https://doi.org/10.1103/PhysRevB.94.214433
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