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research article

Protocols for x-ray transient grating pump/optical probe experiments at x-ray free electron lasers

Fainozzi, Danny
•
Cucini, Riccardo
•
Vila-Comamala, Joan
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September 27, 2024
Journal of Physics B: Atomic, Molecular and Optical Physics

Transient grating spectroscopy is a specialized application of the four-wave-mixing methodology and constitutes a versatile technique for investigating the dynamics of vibrational, magnetic and electronic degrees of freedom of matter in a background-free fashion. Recent developments in free-electron laser sources have enabled the extension of this technique into the extreme ultraviolet range. Ongoing efforts to expand transient grating spectroscopy into the x-ray regime promise numerous advantages: (1) substantial penetration depths that allow for probing bulk material properties, (2) element specificity via specific core-excited states, and (3) short wavelengths that allow for excitation gratings with higher momentum transfer and improved spatial resolution. In this study, we comprehensively outline the procedures for conducting x-ray transient grating pump/optical probe experiment. The process encompasses the design and alignment of the experimental setup, as well as the subsequent steps involved in data acquisition and analysis. This paper is intended as a comprehensive guide for researchers interested in implementing x-ray transient grating spectroscopy, providing valuable insights into the intricacies of the experimental workflow required for this novel technique. Furthermore, we discuss the potential for extending this methodology to an x-ray pump/x-ray probe scheme, envisioning a future direction that holds promise for enhancing the capabilities and scope of x-ray transient grating spectroscopy, opening new opportunities for studying ultrafast processes with unprecedented temporal and spatial resolutions.

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Type
research article
DOI
10.1088/1361-6455/ad717f
Scopus ID

2-s2.0-85203130190

Author(s)
Fainozzi, Danny

University of Bern, Institute of Applied Physics

Cucini, Riccardo

CNR-Istituto Officina dei Materiali

Vila-Comamala, Joan

Paul Scherrer Institut

Lima, Frederico

European XFEL GmbH

Ardana-Lamas, Fernando

European XFEL GmbH

Bañares, Luis

IMDEA Nanociencia

Bargheer, Matias

Institut für Physik

Bencivenga, Filippo

Elettra-Sincrotrone Trieste S.C.p.A.

Berndt, Nadia

Massachusetts Institute of Technology

Beye, Martin

Stockholms universitet

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Date Issued

2024-09-27

Publisher

IOP Publishing

Published in
Journal of Physics B: Atomic, Molecular and Optical Physics
Volume

57

Issue

18

Article Number

185403

Subjects

free electron laser

•

transient grating

•

ultrafast

•

x-ray

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
PH-SB  
FunderFunding(s)Grant NumberGrant URL

Nanoscience Foundry and Fine Analysis

U.S. Department of Energy

NFFA-MUR

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Available on Infoscience
January 24, 2025
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/243763
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