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research article

Ultrarapid crystallization of low-dimensional perovskite with excellent stability for future high-throughput fabrication

Ma, Hongru
•
Chen, Min
•
Wang, Shi
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December 14, 2022
Journal Of Power Sources

Perovskite solar cells (PSCs) as an emerging photovoltaic technique have achieved exceptional power conversion efficiency (PCE) up to 25.7% after fast development over the past decade. But currently some critical issues are still not well addressed in terms of realizing large-scale fabrication, for example, fast fabrication of high-quality perovskite film with good stability. Here, we demonstrate the use of stable and fast-crystallizing low-dimensional (LD) perovskite thin films as the light absorber with only a 10 s annealing time at 250 degrees C, delivering a PCE of 18.16%. The crystallization and photoelectric properties of LD perovskite are well illustrated. The reduction in the annealing time will dramatically increase the productivity of PSCs. The PSCs based on rapidly annealed LD perovskite thin films exhibit excellent stability, with only 12% loss of PCE after 1000 h storage at 85 degrees C and 40-70% relative humidity.

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Type
research article
DOI
10.1016/j.jpowsour.2022.232475
Web of Science ID

WOS:000929733100001

Author(s)
Ma, Hongru
Chen, Min
Wang, Shi
Dong, Qingshun
Zheng, Xiaopeng
Wieliczka, Brian
Luther, Joseph M.
Liu, Xuehui
Zhang, Yi  
Guo, Jingya
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Date Issued

2022-12-14

Publisher

ELSEVIER

Published in
Journal Of Power Sources
Volume

556

Article Number

232475

Subjects

Chemistry, Physical

•

Electrochemistry

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Energy & Fuels

•

Materials Science, Multidisciplinary

•

Chemistry

•

Materials Science

•

perovskite solar cells

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fast crystallizing

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low -dimensional perovskite

•

stability

•

solar-cells

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
GMF  
Available on Infoscience
March 27, 2023
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/196536
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