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  4. Magnetic Field Induced Quantum Spin Liquid in the Two Coupled Trillium Lattices of K2Ni2(SO4)(3)
 
research article

Magnetic Field Induced Quantum Spin Liquid in the Two Coupled Trillium Lattices of K2Ni2(SO4)(3)

Zivkovic, Ivica  
•
Favre, Virgile  
•
Mejia, Catalina Salazar
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October 6, 2021
Physical Review Letters

Quantum spin liquids are exotic states of matter that form when strongly frustrated magnetic interactions induce a highly entangled quantum paramagnet far below the energy scale of the magnetic interactions. Three-dimensional cases are especially challenging due to the significant reduction of the influence of quantum fluctuations. Here, we report the magnetic characterization of K2Ni2(SO4)(3) forming a three-dimensional network of Ni2+ spins. Using density functional theory calculations, we show that this network consists of two interconnected spin-1 trillium lattices. In the absence of a magnetic field, magnetization, specific heat, neutron scattering, and muon spin relaxation experiments demonstrate a highly correlated and dynamic state, coexisting with a peculiar, very small static component exhibiting a strongly renonnalized moment. A magnetic field B greater than or similar to 4 T diminishes the ordered component and drives the system into a pure quantum spin liquid state. This shows that a system of interconnected S = 1 trillium lattices exhibits a significantly elevated level of geometrical frustration.

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Type
research article
DOI
10.1103/PhysRevLett.127.157204
Web of Science ID

WOS:000705651600013

Author(s)
Zivkovic, Ivica  
Favre, Virgile  
Mejia, Catalina Salazar
Jeschke, Harald O.
Magrez, Arnaud  
Dabholkar, Bhupen
Noculak, Vincent
Freitas, Rafael S.
Jeong, Minki
Hegde, Nagabhushan G.  
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Date Issued

2021-10-06

Publisher

AMER PHYSICAL SOC

Published in
Physical Review Letters
Volume

127

Issue

15

Article Number

157204

Subjects

Physics, Multidisciplinary

•

Physics

•

fluctuations

•

transition

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LNNME  
LQM  
Available on Infoscience
November 6, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/182922
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