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  4. Mode-Specific Coupling of Nanoparticle-on-Mirror Cavities with Cylindrical Vector Beams
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research article

Mode-Specific Coupling of Nanoparticle-on-Mirror Cavities with Cylindrical Vector Beams

Vento, Valeria  
•
Roelli, Philippe
•
Verlekar, Sachin  
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May 19, 2023
Nano Letters

Nanocavities formed by ultrathin metallic gaps permitthe reproducibleengineering and enhancement of light-matter interaction, withmode volumes reaching the smallest values allowed by quantum mechanics.While the enhanced vacuum field in metallic nanogaps has been firmlyevidenced, fewer experimental reports have examined the far-fieldto near-field input coupling under strongly focused laser beam. Here,we experimentally demonstrate selective excitation of nanocavity modescontrolled by the polarization and frequency of the laser beam. Wereveal mode selectivity by recording confocal maps of Raman scatteringexcited by cylindrical vector beams, which are compared to the knownexcitation near-field patterns. Our measurements reveal the transversevs longitudinal polarization of the excited antenna mode and how theinput coupling rate depends on laser wavelength. The method introducedhere is easily applicable to other experimental scenarios, and ourresults help connect far-field with near-field parameters in quantitativemodels of nanocavity-enhanced phenomena.

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Type
research article
DOI
10.1021/acs.nanolett.3c00561
Web of Science ID

WOS:001008302400001

Author(s)
Vento, Valeria  
Roelli, Philippe
Verlekar, Sachin  
Galland, Christophe  
Date Issued

2023-05-19

Published in
Nano Letters
Volume

23

Issue

11

Start page

4885

End page

4892

Subjects

Chemistry, Multidisciplinary

•

Chemistry, Physical

•

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Chemistry

•

Science & Technology - Other Topics

•

Materials Science

•

Physics

•

plasmonic cavities

•

plasmonic antennas

•

near-field

•

cylindrical vector beams

•

surface-enhanced raman scattering

•

plasmonic nanocavity modes

•

single-molecule

•

room-temperature

•

induced transparency

•

optomechanics

•

enhancement

•

field

•

emission

•

spectroscopy

•

absorption

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQNO
Available on Infoscience
July 17, 2023
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/199115
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