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  4. Triplons, magnons, and spinons in a single quantum spin system: SeCuO3
 
research article

Triplons, magnons, and spinons in a single quantum spin system: SeCuO3

Testa, Luc  
•
Surija, Vinko
•
Prsa, Krunoslav
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January 25, 2021
Physical Review B

Quantum magnets display a wide variety of collective excitations, including spin waves (magnons), coherent singlet-triplet excitations (triplons), and pairs of fractional spins (spinons). These modes differ radically in nature and properties, and in all conventional analyses any given material is interpreted in terms of only one type. We report inelastic neutron scattering measurements on the spin-1/2 antiferromagnet SeCuO3, which demonstrate that this compound exhibits all three primary types of spin excitation. Cu-2 sites form strongly bound dimers while Cu-2 sites form a network of spin chains, whose weak three-dimensional (3D) coupling induces antiferromagnetic order. We perform quantitative modeling to extract all of the relevant magnetic interactions and show that magnons of the Cu-2 system give a lower bound to the spinon continua, while the Cu-2 system hosts a band of high-energy triplons at the same time as frustrating the 3D network.

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Type
research article
DOI
10.1103/PhysRevB.103.L020409
Web of Science ID

WOS:000611675300009

Author(s)
Testa, Luc  
Surija, Vinko
Prsa, Krunoslav
Steffens, Paul
Boehm, Martin
Bourges, Philippe
Berger, Helmuth  
Normand, Bruce  
Ronnow, Henrik M.  
Zivkovic, Ivica  
Date Issued

2021-01-25

Publisher

AMER PHYSICAL SOC

Published in
Physical Review B
Volume

103

Issue

2

Article Number

L020409

Subjects

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Materials Science

•

Physics

•

magnetic-properties

•

crystal-structures

•

bound-states

•

excitations

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

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Available on Infoscience
March 26, 2021
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/176793
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