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research article

Self-organized spatiotemporal quasi-phase-matching in microresonators

Zhou, J.  
•
Hu, Jianqi  
•
Clementi, Marco  
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May 1, 2025
Nature Communications

Quasi-phase-matching (QPM) is a widely adopted technique for mitigating stringent momentum conservation in nonlinear optical processes such as second-harmonic generation (SHG). It effectively compensates for the phase velocity mismatch between optical harmonics by introducing a periodic spatial modulation to the nonlinear optical medium. Such a mechanism has been further generalized to the spatiotemporal domain, where a non-stationary spatial QPM can induce a frequency shift of the generated light. Here we demonstrate how a spatiotemporal QPM grating, consisting in a concurrent spatial and temporal modulation of the nonlinear response, naturally emerges through all-optical poling in silicon nitride microresonators. Mediated by the coherent photogalvanic effect, a traveling space-charge grating is self-organized, affecting momentum and energy conservation, resulting in a quasi-phase-matched and Doppler-shifted second harmonic. Our observation of the photoinduced spatiotemporal QPM expands the scope of phase matching conditions in nonlinear photonics.

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10.1038_s41467-025-59215-1.pdf

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Main Document

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http://purl.org/coar/version/c_970fb48d4fbd8a85

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openaccess

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CC BY

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1.45 MB

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3a6a52406824cf94a59bde1354018d17

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