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research article

Evolution of magnetic and crystal structures in the multiferroic FeTe2O5Br

Pregelj, M.
•
Jeglic, P.
•
Zorko, A.
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2013
Physical Review B

Neutron diffraction and nuclear quadrupole resonance (NQR) measurements were employed to investigate magnetic order in the nonferroelectric phase preceding the low-temperature multiferroic state in FeTe2O5Br. Refinement of the neutron diffraction data and simulations of Br-79,Br-81 NQR spectra reveal that the incommensurate magnetic ordering in the nonferroelectric state comprises amplitude-modulated magnetic moments, similar to that seen in the multiferroic state. The two ordered states differ in the orientation of the magnetic moments and phase shifts between modulation waves. Surprisingly, all symmetry restrictions for the electric polarization are absent in both states. The different ferroelectric responses of the two states are thus argued to arise from the differences in the phase shifts between certain modulation waves, which cancel out in the nonferrolectric state. DOI: 10.1103/PhysRevB.87.144408

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Type
research article
DOI
10.1103/PhysRevB.87.144408
Web of Science ID

WOS:000317391200006

Author(s)
Pregelj, M.
Jeglic, P.
Zorko, A.
Zaharko, O.
Apih, T.
Gradisek, A.
Komelj, M.
Berger, H.  
Arcon, D.
Date Issued

2013

Publisher

American Physical Society

Published in
Physical Review B
Volume

87

Issue

14

Article Number

144408

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSE  
Available on Infoscience
October 1, 2013
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/95074
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