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  4. Spin Correlations and Short-Range Magnetic Order in the Honeycomb-Layered Na2Ni2TeO6
 
research article

Spin Correlations and Short-Range Magnetic Order in the Honeycomb-Layered Na2Ni2TeO6

Korshunov, Artem
•
Safiulina, Irina  
•
Kurbakov, Alexander
March 1, 2020
Physica Status Solidi B-Basic Solid State Physics

An experimental study of long-range magnetic order formation mechanisms in a layered structure with a honeycomb arrangement of the magnetic atoms Na2Ni2TeO6 is conducted. For the first time, the strong spin correlations are directly observed above the Neel temperature T-N that is manifested in the presence of broad diffuse peaks on neutron diffraction patterns obtained with the XYZ polarization analysis. Due to the possibility of separating the magnetic, nuclear incoherent, and nuclear coherent contributions to the total neutron scattering cross section, it is unequivocally established that the observed diffuse scattering has magnetic nature. The spin-pair correlation function is reconstructed by modeling diffuse neutron scattering on Na2Ni2TeO6 with reverse Monte Carlo method. The obtained results indicate 2D nature of the magnetic correlations, and moreover, the symmetry of short-range magnetic state corresponds to long-range zigzag-type magnetic order in the honeycomb net, which is established earlier based on the theoretical calculations.

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Type
research article
DOI
10.1002/pssb.201900232
Web of Science ID

WOS:000519218800022

Author(s)
Korshunov, Artem
Safiulina, Irina  
Kurbakov, Alexander
Date Issued

2020-03-01

Publisher

WILEY-V C H VERLAG GMBH

Published in
Physica Status Solidi B-Basic Solid State Physics
Volume

257

Issue

3

Article Number

1900232

Subjects

Physics, Condensed Matter

•

Physics

•

diffuse magnetic scattering

•

honeycomb structure

•

magnetism

•

neutron scattering

•

magnetoresistance

•

antiferromagnet

•

scattering

•

lattice

•

phase

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
Available on Infoscience
March 26, 2020
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/167669
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