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  4. Doping evolution of the oxygen K-edge x-ray absorption spectra of cuprate superconductors using a three-orbital Hubbard model
 
research article

Doping evolution of the oxygen K-edge x-ray absorption spectra of cuprate superconductors using a three-orbital Hubbard model

Chen, C. -C.
•
Sentef, M.
•
Kung, Y. F.
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2013
Physical Review B

We study oxygen K-edge x-ray absorption spectroscopy (XAS) and investigate the validity of the Zhang-Rice singlet (ZRS) picture in overdoped cuprate superconductors. Using large-scale exact diagonalization of the three-orbital Hubbard model, we observe the effect of strong correlations manifesting in a dynamical spectral weight transfer from the upper Hubbard band to the ZRS band. The quantitative agreement between theory and experiment highlights an additional spectral weight reshuffling due to core-hole interaction. Our results confirm the important correlated nature of the cuprates and elucidate the changing orbital character of the low-energy quasiparticles, but also demonstrate the continued relevance of the ZRS even in the overdoped region.

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Type
research article
DOI
10.1103/PhysRevB.87.165144
Web of Science ID

WOS:000318520900008

Author(s)
Chen, C. -C.
Sentef, M.
Kung, Y. F.
Jia, C. J.
Thomale, R.
Moritz, B.
Kampf, A. P.
Devereaux, T. P.
Date Issued

2013

Publisher

Amer Physical Soc

Published in
Physical Review B
Volume

87

Issue

16

Article Number

165144

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
ITP  
Available on Infoscience
October 1, 2013
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/95473
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