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  4. Magnetic structure of the two-dimensional XY antiferromagnet Sr2CoSi2O7 studied using single-crystal neutron diffraction
 
research article

Magnetic structure of the two-dimensional XY antiferromagnet Sr2CoSi2O7 studied using single-crystal neutron diffraction

Dutta, Rajesh
•
Thoma, Henrik
•
Sazonov, Andrew
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January 25, 2023
Physical Review B

We report a combined polarized and unpolarized neutron diffraction study on a multiferroic Sr2CoSi2O7 (SCSO) single crystal below and above the antiferromagnetic ordering temperature TN = 6.5 K. Unpolarized neutron diffraction measurements at 15 K confirm the melilite-type tetragonal P4 over bar 21m space group as the parent structure of SCSO. The low temperature study at 2.3 K, in contrast, reveals symmetry lowering with the orthorhombic Cmm'2' and P212'12' magnetic space groups being equally possible. In these Cmm'2' and P212'12' magnetic space groups we obtain a very similar ordered magnetic moment about 2.86 and 2.94 mu B/Co2+, respectively, which lies in the ab plane. Our spin polarized flipping ratio measurements under an applied magnetic field of 6 T in the paramagnetic state support the results of our bulk magnetization data, indicating strong easy-plane spin anisotropy, responsible for the in-plane order below TN.

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Type
research article
DOI
10.1103/PhysRevB.107.014420
Web of Science ID

WOS:000927608900003

Author(s)
Dutta, Rajesh
Thoma, Henrik
Sazonov, Andrew
Nafradi, Balint  
Meven, Martin
Gukasov, Arsen
Kocsis, Vilmos
Zeitler, Uli
Puri, Alessandro
Tokunaga, Yusuke
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Date Issued

2023-01-25

Publisher

AMER PHYSICAL SOC

Published in
Physical Review B
Volume

107

Issue

1

Article Number

014420

Subjects

Materials Science, Multidisciplinary

•

Physics, Applied

•

Physics, Condensed Matter

•

Materials Science

•

Physics

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LPMC  
Available on Infoscience
March 13, 2023
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/195896
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