Repository logo

Infoscience

  • English
  • French
Log In
Logo EPFL, École polytechnique fédérale de Lausanne

Infoscience

  • English
  • French
Log In
  1. Home
  2. Academic and Research Output
  3. Journal articles
  4. Anomalous spin dynamics in the coupled spin tetramer system CuSeO3
 
research article

Anomalous spin dynamics in the coupled spin tetramer system CuSeO3

Lee, S.
•
Lee, W. -J.
•
Van Tol, J.
Show more
2017
Physical Review B

We report high-field magnetization, high-frequency electron spin resonance (ESR), and Se-77 nuclear magnetic resonance (NMR) measurements on the linear spin tetramer system CuSeO3, consisting of strongly interacting Cu(1) dimers and weakly coupled Cu(2) spins. The magnetization exhibits anisotropic half-step magnetization plateaus at mu H-0 = 45 T, depending on a crystallographic orientation. A temperature dependence of the ESR linewidth Delta H-pp in a paramagnetic phase points towards the significance of anisotropic exchange interactions. Below T-N = 9-10 K long-range magnetic order is evidenced by the observation of a critical divergence of both Delta H-pp(T) and the nuclear spin-lattice relaxation rate 1/T-1. In addition, we identify a magnetic anomaly at T* = 6.0(5) K below T-N, which is caused by a spin reorientation. The nuclear spin-spin relaxation rate 1/T-2 unveils the development of site-specific spin correlations. The intriguing magnetism of CuSeO3 is discussed in terms of the energy hierarchy of Cu(1) and Cu(2) spins in concert with additional intertetramer interactions.

  • Details
  • Metrics
Type
research article
DOI
10.1103/PhysRevB.95.054405
Web of Science ID

WOS:000397639200002

Author(s)
Lee, S.
•
Lee, W. -J.
•
Van Tol, J.
•
Kuhns, P. L.
•
Reyes, A. P.
•
Berger, H.  
•
Choi, K. -Y.
Date Issued

2017

Publisher

Amer Physical Soc

Published in
Physical Review B
Volume

95

Issue

5

Article Number

054405

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LSE  
Available on Infoscience
May 1, 2017
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/136946
Logo EPFL, École polytechnique fédérale de Lausanne
  • Contact
  • infoscience@epfl.ch

  • Follow us on Facebook
  • Follow us on Instagram
  • Follow us on LinkedIn
  • Follow us on X
  • Follow us on Youtube
AccessibilityLegal noticePrivacy policyCookie settingsEnd User AgreementGet helpFeedback

Infoscience is a service managed and provided by the Library and IT Services of EPFL. © EPFL, tous droits réservés