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research article

Generation and control of localized terahertz fields in photoemitted electron plasmas

Dias, Eduardo J. C.
•
Madan, Ivan  
•
Gargiulo, Simone  
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May 4, 2023
Nanoscale Advances

Dense micron-sized electron plasmas, such as those generated upon irradiation of nanostructured metallic surfaces by intense femtosecond laser pulses, constitute a rich playground to study light-matter interactions, many-body phenomena, and out-of-equilibrium charge dynamics. Besides their fundamental interest, laser-induced plasmas hold great potential for the generation of localized terahertz radiation pulses. However, the underlying mechanisms ruling the formation and evolution of such plasmas are not yet well understood. Here, we develop a comprehensive microscopic theory to predictably describe the spatiotemporal dynamics of laser-pulse-induced plasmas. Through detailed analysis of electron emission, metal screening, and plasma cloud interactions, we investigate the spatial, temporal, and spectral characteristics of the so-generated terahertz fields, which can be extensively controlled through the metal morphology and the illumination conditions. We further describe the interaction with femtosecond electron beams to explain recent ultrafast electron microscopy experiments, whereby the position and temporal dependence of the observed electron acceleration permits assessing the associated terahertz field. Besides its potential application to the design of low-frequency light sources, our work contributes fundamental insight into the generation and dynamics of micron-scale electron plasmas and their interaction with ultrafast electron pulses.

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Type
research article
DOI
10.1039/d3na00168g
Web of Science ID

WOS:001006416500001

Author(s)
Dias, Eduardo J. C.
Madan, Ivan  
Gargiulo, Simone  
Barantani, Francesco  
Yannai, Michael
Vanacore, Giovanni Maria  
Kaminer, Ido
Carbone, Fabrizio  
de Abajo, F. Javier Garcia
Date Issued

2023-05-04

Publisher

ROYAL SOC CHEMISTRY

Published in
Nanoscale Advances
Subjects

Chemistry, Multidisciplinary

•

Nanoscience & Nanotechnology

•

Materials Science, Multidisciplinary

•

Chemistry

•

Science & Technology - Other Topics

•

Materials Science

•

optical rectification

•

spectroscopy

•

microscopy

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LUMES  
Available on Infoscience
July 3, 2023
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/198757
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