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research article

Controlling the nonlinear optical properties of plasmonic nanoparticles with the phase of their linear response

Butet, Jeremy
•
Raziman, T. V.
•
Yang, Kuang-Yu  
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2016
Optics Express

We numerically investigate the second harmonic generation from different plasmonic systems and evidence the key role played in their nonlinear response by the phase at the fundamental wavelength. In the case of a single plasmonic nanorod, the interference between the second harmonic dipolar and quadrupolar emission modes depends on their relative phase, which is deeply related to the excitation wavelength. The knowledge obtained in this simple case is then used to describe and understand the nonlinear response from a more complex structure, namely a gold nanodolmen. The complex phase evolution associated with a Fano resonance arising at the fundamental wavelength enables dramatically modifying the second harmonic emission patterns from plasmonic metamolecules within minute wavelength shifts. These results emphasize the importance of the phase in the nonlinear optical processes arising in plasmonic nanostructures, in addition to the increase in conversion yield associated with the excitation of localized surface plasmon resonances. (C) 2016 Optical Society of America

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Type
research article
DOI
10.1364/Oe.24.017138
Web of Science ID

WOS:000384715800090

Author(s)
Butet, Jeremy
Raziman, T. V.
Yang, Kuang-Yu  
Bernasconi, Gabriel D.
Martin, O. J. F.  
Date Issued

2016

Publisher

Optical Society of America

Published in
Optics Express
Volume

24

Issue

15

Start page

17138

End page

17148

Subjects

Nanophotonics

•

Plasmonics

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
NAM  
Available on Infoscience
November 21, 2016
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/131280
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