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research article

Electrical and Magnetic Properties of FeGa3 with Antisite Disorder

Ribeiro, C. Kaufmann
•
Rabello, A. Faé
•
Martelli, V.
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December 1, 2023
New Physics: Sae Mulli

We investigated the electronic and magnetic ground states of the cage compound FeGa3 under the presence of Fe antisite disorder (namely as Fe0.258Ga0.742) by x-ray diffraction (XRD), Mössbauer spectroscopy (MS), magnetization and electrical resistivity. Our results show that approximately 4.5 (5)% Fe antisite occupying one of the two non-equivalent Ga sites changes significantly the electronic and magnetic ground states of the pristine compound. We uncover that Fe0.258Ga0.742 undergoes two magnetic transitions, T1 ≈ 60 K and T2 ≈ 15 K, the latter associated with the suppression of semiconducting behavior. We focus our discussion on the role that in-gap impurity states and spin disorder play across semiconducting-metal and paramagnetic-magnetic transitions.

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Type
research article
DOI
10.3938/NPSM.73.1149
Scopus ID

2-s2.0-85181255655

Author(s)
Ribeiro, C. Kaufmann
Rabello, A. Faé
Martelli, V.
Zivkovic, I.  

École Polytechnique Fédérale de Lausanne

Fogh, E.  

École Polytechnique Fédérale de Lausanne

Rønnow, H. M.  

École Polytechnique Fédérale de Lausanne

Cornejo, D.
Jiménez, J. Larrea
Date Issued

2023-12-01

Published in
New Physics: Sae Mulli
Volume

73

Issue

12

Start page

1149

End page

1154

Subjects

Condensed Matter Physics

•

Narrow-band semiconductors

•

Strongly correlated electron systems

Editorial or Peer reviewed

REVIEWED

Written at

EPFL

EPFL units
LQM  
FunderFunding(s)Grant NumberGrant URL

M.C.A. Fantini

Los Alamos National Laboratory

European Research Council

810451

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Available on Infoscience
January 16, 2025
Use this identifier to reference this record
https://infoscience.epfl.ch/handle/20.500.14299/242846
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